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qp_plugins_scemama/devel/density_matrix/density_matrix_array.irp.f

116 lines
3.8 KiB
Fortran

use bitmasks
BEGIN_PROVIDER [ double precision, two_e_dm_aa, (mo_num,mo_num,mo_num,mo_num) ]
&BEGIN_PROVIDER [ double precision, two_e_dm_bb, (mo_num,mo_num,mo_num,mo_num) ]
&BEGIN_PROVIDER [ double precision, two_e_dm_ab, (mo_num,mo_num,mo_num,mo_num) ]
implicit none
use bitmasks
BEGIN_DOC
! Temporary files for 2-e dm calculation
END_DOC
integer :: getUnitAndOpen
integer :: k,l,degree, idx,i,j
integer :: exc(0:2,2,2),n_occ_alpha
double precision :: phase, coef
integer :: h1,h2,p1,p2,s1,s2, e1, e2
double precision :: ck, cl
character*(128), parameter :: f = '(i8,4(x,i5),x,d16.8)'
integer :: istate
two_e_dm_aa = 0.d0
two_e_dm_ab = 0.d0
two_e_dm_bb = 0.d0
istate = 1
! OMP PARALLEL DEFAULT(SHARED) PRIVATE(k,ck,ckl,i,j,e1,e2,cl,phase,h1,p1,h2,p2,s1,s2,occ)
! OMP DO SCHEDULE(dynamic,64)
do k=1,N_det
ck = psi_coef(k,istate)
call bitstring_to_list(psi_det(1,1,k), occ(1,1), n_occ_alpha, N_int)
call bitstring_to_list(psi_det(1,2,k), occ(1,2), n_occ_alpha, N_int)
ckl = psi_coef(k,istate) * psi_coef(k,istate)
do i = 1,elec_alpha_num
e1=occ(i,1)
do j = 1,elec_alpha_num
e2=occ(j,1)
! alpha-alpha
two_e_dm_aa(e1,e2,e1,e2) += 0.5d0*ckl
two_e_dm_aa(e1,e2,e2,e1) -= 0.5d0*ckl
enddo
do j = 1,elec_beta_num
e2=occ(j,2)
! alpha-beta
two_e_dm_ab(e1,e2,e1,e2) += ckl
enddo
enddo
do i = 1,elec_beta_num
e1=occ(i,2)
do j = 1,elec_beta_num
e2=occ(j,2)
! beta-beta
two_e_dm_bb(e1,e2,e1,e2) += 0.5d0*ckl
two_e_dm_bb(e1,e2,e2,e1) -= 0.5d0*ckl
enddo
enddo
do l=1,k-1
cl = 2.d0*psi_coef(l,istate)
call get_excitation_degree(psi_det(1,1,k),psi_det(1,1,l),degree,N_int)
if (degree == 2) then
call get_double_excitation(psi_det(1,1,k),psi_det(1,1,l),exc,phase,N_int)
call decode_exc(exc,degree,h1,p1,h2,p2,s1,s2)
ckl = phase*ck*cl
select case (s1+s2)
case(2) ! alpha alpha
two_e_dm_aa(h1,h2,p1,p2) += ckl
two_e_dm_aa(h1,h2,p2,p1) -= ckl
case(3) ! alpha beta
two_e_dm_ab(h1,h2,p1,p2) += ckl
case(4) ! beta beta
two_e_dm_bb(h1,h2,p1,p2) += ckl
two_e_dm_bb(h1,h2,p2,p1) -= ckl
end select
else if (degree == 1) then
call get_single_excitation(psi_det(1,1,k),psi_det(1,1,l),exc,phase,N_int)
call decode_exc(exc,degree,h1,p1,h2,p2,s1,s2)
double precision :: ckl
ckl = phase*ck*cl
call bitstring_to_list(psi_det(1,1,k), occ(1,1), n_occ_alpha, N_int)
call bitstring_to_list(psi_det(1,2,k), occ(1,2), n_occ_alpha, N_int)
select case (s1)
case (1) ! Alpha single excitation
integer :: occ(N_int*bit_kind_size,2)
do i = 1, elec_alpha_num
p2=occ(i,1)
h2=p2
two_e_dm_aa(h1,h2,p1,p2) += ckl
two_e_dm_aa(h1,h2,p2,p1) -= ckl
enddo
do i = 1, elec_beta_num
p2=occ(i,2)
h2=p2
two_e_dm_ab(h1,h2,p1,p2) += ckl
enddo
case (2) ! Beta single excitation
do i = 1, elec_alpha_num
p2=occ(i,1)
h2=p2
two_e_dm_ab(h1,h2,p1,p2) += ckl
enddo
do i = 1, elec_beta_num
p2=occ(i,2)
h2=p2
two_e_dm_bb(h1,h2,p1,p2) += ckl
two_e_dm_bb(h1,h2,p2,p1) -= ckl
enddo
end select
endif
enddo
enddo
! OMP END DO
! OMP END PARALLEL
END_PROVIDER