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qp_plugins_scemama/stable/amplitudes/extract_amplitudes.irp.f
2019-09-11 17:09:30 +02:00

248 lines
7.5 KiB
Fortran

program extract_amplitudes
implicit none
BEGIN_DOC
! Print the T1 and T2 amplitudes into a file.
END_DOC
read_wf = .True.
TOUCH read_wf
call run
end
subroutine run
implicit none
BEGIN_DOC
! Compute t1 and T2 amplitudes
END_DOC
double precision, allocatable :: t1_a(:,:), t1_b(:,:)
double precision, allocatable :: t2_aa(:,:,:,:)
double precision, allocatable :: t2_ab(:,:,:,:)
double precision, allocatable :: t2_bb(:,:,:,:)
double precision :: phase, norm
integer :: exc(0:2,2,2), degree
integer :: h1,h2,p1,p2,s1,s2, istate
integer :: i,j,k,l,a,b,c,d
character*(32) :: buffer
call getenv('QP_STATE',buffer)
istate = 1
read(buffer,*,err=5,end=5) istate
5 continue
call write_int(6,istate,'State for amplitudes')
allocate ( &
t1_a(elec_alpha_num,mo_num), &
t1_b(elec_alpha_num,mo_num), &
t2_aa(elec_alpha_num,elec_alpha_num,mo_num,mo_num), &
t2_ab(elec_alpha_num,elec_alpha_num,mo_num,mo_num), &
t2_bb(elec_alpha_num,elec_alpha_num,mo_num,mo_num) )
t1_a = 0.d0
t1_b = 0.d0
t2_aa = 0.d0
t2_ab = 0.d0
t2_bb = 0.d0
integer :: i_ref
i_ref = maxloc( dabs(psi_coef(:,istate)), dim=1 )
norm = 1.d0 / psi_coef(i_ref,istate)
do k=1,N_det
call get_excitation_degree(psi_det(1,1,i_ref),psi_det(1,1,k),degree,N_int)
select case (degree)
case (1)
call get_excitation(psi_det(1,1,i_ref),psi_det(1,1,k),exc,degree,phase,N_int)
call decode_exc(exc,degree,h1,p1,h2,p2,s1,s2)
if (h1 > elec_alpha_num) then
print *, irp_here, "h1 > elec_alpha_num"
endif
if (p1 <= elec_alpha_num) then
print *, irp_here, "p1 <= elec_alpha_num"
endif
if (s1 == 1) then
t1_a(h1,p1) += phase * psi_coef(k,istate) * norm
else if (s1 == 2) then
t1_b(h1,p1) += phase * psi_coef(k,istate) * norm
else
print *, irp_here, ': Bug!', s1, s2
endif
case (2)
call get_excitation(psi_det(1,1,i_ref),psi_det(1,1,k),exc,degree,phase,N_int)
call decode_exc(exc,degree,h1,p1,h2,p2,s1,s2)
if (h1 > elec_alpha_num) then
print *, irp_here, "h1 > elec_alpha_num"
endif
if (p1 <= elec_alpha_num) then
print *, irp_here, "p1 <= elec_alpha_num"
endif
if (h2 > elec_alpha_num) then
print *, irp_here, "h2 > elec_alpha_num"
endif
if (p2 <= elec_alpha_num) then
print *, irp_here, "p2 <= elec_alpha_num"
endif
if ( (s1 == 1).and.(s2 == 1) ) then
t2_aa(h1,h2,p1,p2) += phase * psi_coef(k,istate) * norm
t2_aa(h1,h2,p2,p1) -= phase * psi_coef(k,istate) * norm
t2_aa(h2,h1,p2,p1) += phase * psi_coef(k,istate) * norm
t2_aa(h2,h1,p1,p2) -= phase * psi_coef(k,istate) * norm
else if ( (s1 == 1).and.(s2 == 2) ) then
t2_ab(h1,h2,p1,p2) += phase * psi_coef(k,istate) * norm * 0.5d0
t2_ab(h2,h1,p2,p1) += phase * psi_coef(k,istate) * norm * 0.5d0
else if ( (s1 == 2).and.(s2 == 1) ) then
print *, irp_here, ': Bug!'
stop -1
else if ( (s1 == 2).and.(s2 == 2) ) then
t2_bb(h1,h2,p1,p2) += phase * psi_coef(k,istate) * norm
t2_bb(h1,h2,p2,p1) -= phase * psi_coef(k,istate) * norm
t2_bb(h2,h1,p2,p1) += phase * psi_coef(k,istate) * norm
t2_bb(h2,h1,p1,p2) -= phase * psi_coef(k,istate) * norm
else
print *, irp_here, ': Bug!'
stop -2
endif
end select
enddo
do b=elec_alpha_num+1, mo_num
do a=elec_alpha_num+1, mo_num
do j=1,elec_alpha_num
do i=1,elec_alpha_num
if ( (i == j).or.(a == b)) then
t2_aa(i,j,a,b) = 0.d0
t2_bb(i,j,a,b) = 0.d0
else
t2_aa(i,j,a,b) -= t1_a(i,a)*t1_a(j,b)
t2_bb(i,j,a,b) -= t1_b(i,a)*t1_b(j,b)
t2_aa(i,j,a,b) += t1_a(i,b)*t1_a(j,a)
t2_bb(i,j,a,b) += t1_b(i,b)*t1_b(j,a)
endif
t2_ab(i,j,a,b) -= 0.5d0* (t1_a(i,a)*t1_b(j,b) + t1_b(i,a)*t1_a(j,b))
enddo
enddo
enddo
enddo
integer :: iunit, getunitandopen
iunit = getunitandopen('t1','w')
write(iunit,*) '# T1_a'
do i=1,elec_alpha_num
do a=elec_alpha_num+1, mo_num
if (t1_a(i,a) /= 0.d0) then
write(iunit,'(I4,X,I4,X,E20.10)') i, a, t1_a(i,a)
endif
enddo
enddo
write(iunit,*) '# T1_b'
do i=1,elec_alpha_num
do a=elec_alpha_num+1, mo_num
if (t1_b(i,a) /= 0.d0) then
write(iunit,'(I4,X,I4,X,E20.10)') i, a, t1_b(i,a)
endif
enddo
enddo
iunit = getunitandopen('t2','w')
write(iunit,*) '# T2_aa'
do i=1,elec_alpha_num
do j=1,elec_alpha_num
do a=elec_alpha_num+1, mo_num
do b=elec_alpha_num+1, mo_num
if (t2_aa(i,j,a,b) /= 0.d0) then
write(iunit,'(4(I4,X),E20.10)') i, j, a, b, t2_aa(i,j,a,b)
endif
enddo
enddo
enddo
enddo
write(iunit,*) '# T2_bb'
do i=1,elec_alpha_num
do j=1,elec_alpha_num
do a=elec_alpha_num+1, mo_num
do b=elec_alpha_num+1, mo_num
if (t2_bb(i,j,a,b) /= 0.d0) then
write(iunit,'(4(I4,X),E20.10)') i, j, a, b, t2_bb(i,j,a,b)
endif
enddo
enddo
enddo
enddo
write(iunit,*) '# T2_ab'
do i=1,elec_alpha_num
do j=1,elec_alpha_num
do a=elec_alpha_num+1, mo_num
do b=elec_alpha_num+1, mo_num
if (t2_ab(i,j,a,b) /= 0.d0) then
write(iunit,'(4(I4,X),E20.10)') i, j, a, b, t2_ab(i,j,a,b)
endif
enddo
enddo
enddo
enddo
double precision :: E0, e_cor
double precision, external :: get_two_e_integral
e_cor = 0.d0
do b=elec_alpha_num+1, mo_num
do j=1,elec_alpha_num
! TODO : singles contributions
! do k=1,mo_num
! e_cor = e_cor + t1_a(j,b) * get_two_e_integral(k,j,k,b,mo_integrals_map)
! e_cor = e_cor + t1_b(j,b) * get_two_e_integral(k,j,k,b,mo_integrals_map)
! enddo
do a=elec_alpha_num+1, mo_num
do i=1,elec_alpha_num
e_cor = e_cor + 0.25d0*( &
t2_aa(i,j,a,b) + t2_bb(i,j,a,b) + &
t1_a(i,a) * t1_a(j,b) + &
t1_b(i,a) * t1_b(j,b) - &
t1_a(i,b) * t1_a(j,a) - &
t1_b(i,b) * t1_b(j,a) &
) * ( &
get_two_e_integral(i,j,a,b,mo_integrals_map) - &
get_two_e_integral(i,j,b,a,mo_integrals_map) )
e_cor = e_cor + 1.0d0 * ( &
t2_ab(i,j,a,b) + &
t1_a(i,a) * t1_b(j,b) ) * &
get_two_e_integral(i,j,a,b,mo_integrals_map)
enddo
enddo
enddo
enddo
e_cor = e_cor
double precision, external :: diag_h_mat_elem
E0 = diag_h_mat_elem(psi_det(1,1,i_ref),N_int) + nuclear_repulsion
print '(A,F15.10)', 'E0 : ', E0
print '(A,F15.10)', 'corr energy: ', e_cor
print '(A,F15.10)', 'total energy: ', E0 + e_cor
deallocate(t1_a,t1_b,t2_aa,t2_ab,t2_bb)
end