From 9148783e138ceec3f3104da48f36072e449abf86 Mon Sep 17 00:00:00 2001 From: =?UTF-8?q?Micka=C3=ABl=20V=C3=A9ril?= Date: Mon, 15 Jun 2020 16:13:03 +0200 Subject: [PATCH] Add graphical abstract support --- config.toml | 2 +- content/publications.html | 4 ++-- static/css/publi.css | 6 ++++++ .../10/1021/acs/jctc/0c00227/abstract.html | 1 + .../10/1021/acs/jctc/0c00227/picture.jpeg | Bin 0 -> 182766 bytes .../10/1021/acs/jctc/8b00406/abstract.html | 1 + .../10/1021/acs/jctc/8b00406/picture.jpeg} | Bin .../10/1021/acs/jctc/8b01205/abstract.html | 1 + .../10/1021/acs/jctc/8b01205/picture.jpeg | Bin 0 -> 127626 bytes .../10/1021/acs/jctc/9b01216/abstract.html | 1 + .../10/1021/acs/jctc/9b01216/picture.jpeg | Bin 0 -> 67466 bytes .../10/1021/acs/jpclett/0c00014/abstract.html | 1 + .../10/1021/acs/jpclett/0c00014/picture.jpeg | Bin 0 -> 118884 bytes static/data/{publis.yaml => publis/index.yaml} | 0 static/js/createPubliUI.js | 17 ++++++++++++++++- static/js/getPublis.js | 2 +- 16 files changed, 31 insertions(+), 5 deletions(-) create mode 100644 static/data/publis/10/1021/acs/jctc/0c00227/abstract.html create mode 100644 static/data/publis/10/1021/acs/jctc/0c00227/picture.jpeg create mode 100644 static/data/publis/10/1021/acs/jctc/8b00406/abstract.html rename static/{img/montain.jpeg => data/publis/10/1021/acs/jctc/8b00406/picture.jpeg} (100%) create mode 100644 static/data/publis/10/1021/acs/jctc/8b01205/abstract.html create mode 100644 static/data/publis/10/1021/acs/jctc/8b01205/picture.jpeg create mode 100644 static/data/publis/10/1021/acs/jctc/9b01216/abstract.html create mode 100644 static/data/publis/10/1021/acs/jctc/9b01216/picture.jpeg create mode 100644 static/data/publis/10/1021/acs/jpclett/0c00014/abstract.html create mode 100644 static/data/publis/10/1021/acs/jpclett/0c00014/picture.jpeg rename static/data/{publis.yaml => publis/index.yaml} (100%) diff --git a/config.toml b/config.toml index 578f344f..11b927c8 100644 --- a/config.toml +++ b/config.toml @@ -8,7 +8,7 @@ theme = "beautifulhugo" # homeTitle = "" subtitle = "QUantum Excited STates database" [[Params.bigimg]] - src = "img/montain.jpeg" + src = "data/publis/10/1021/acs/jctc/8b00406/picture.jpeg" desc = "A mountaineering analogy of the QUEST project" [markup] [markup.goldmark] diff --git a/content/publications.html b/content/publications.html index 0080e055..c50ecbfd 100644 --- a/content/publications.html +++ b/content/publications.html @@ -26,7 +26,7 @@ draft: false const uospublis = spubliscite.format('data', { format: 'object' }) const spublis = uospublis.sort((puba,pubb)=>pubUtils.getIssuedDate(puba) - pubUtils.getIssuedDate(pubb)) for (const publi of spublis) { - art=createPubliUI(publi,pubs.sets,true) + art= await createPubliUI(publi,pubs.sets,true,true) $(art).appendTo("#publis_sets") } const odois=Array.from(pubs.others.keys()) @@ -34,7 +34,7 @@ draft: false const uoopublis = opubliscite.format('data', { format: 'object' }) const opublis = uoopublis.sort((puba,pubb)=>pubUtils.getIssuedDate(puba) - pubUtils.getIssuedDate(pubb)) for (const publi of opublis) { - art=createPubliUI(publi,pubs.others,true) + art= await createPubliUI(publi,pubs.others,true,true) $(art).appendTo("#publis_others") } } diff --git a/static/css/publi.css b/static/css/publi.css index b8ed845f..5ef68c6f 100644 --- a/static/css/publi.css +++ b/static/css/publi.css @@ -11,6 +11,12 @@ padding: 0; border: 0 } +.publi .abstract > figure.picture{ + width: 60%; + padding: 0px; + margin: 10px; + float: right; +} .publi ul.authors-list li.author-item{ display: inline; diff --git a/static/data/publis/10/1021/acs/jctc/0c00227/abstract.html b/static/data/publis/10/1021/acs/jctc/0c00227/abstract.html new file mode 100644 index 00000000..5436b66f --- /dev/null +++ b/static/data/publis/10/1021/acs/jctc/0c00227/abstract.html @@ -0,0 +1 @@ +Aiming at completing the sets of FCI-quality transition energies that we recently developed (J. Chem. Theory Comput.2018, 14, 4360–4379, ibid.2019, 15, 1939–1956, and ibid.2020, 16, 1711–1741), we provide, in the present contribution, ultra-accurate vertical excitation energies for a series of “exotic” closed-shell molecules containing F, Cl, P, and Si atoms and small radicals, such as CON and its variants, that were not considered to date in such investigations. This represents a total of 81 high-quality transitions obtained with a series of diffuse-containing basis sets of various sizes. For the exotic compounds, these transitions are used to perform benchmarks with a vast array of lower level models, i.e., CIS(D), EOM-MP2, (SOS/SCS)-CC2, STEOM-CCSD, CCSD, CCSDR(3), CCSDT-3, (SOS-)ADC(2), and ADC(3). Additional comparisons are made with literature data. 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In this way, we define a list of 110 transition energies for states of various characters (valence, Rydberg, n → π*, π → π*, singlet, triplet, etc.) to be used as references for further calculations. Benchmark transition energies are provided at the aug-cc-pVTZ level as well as with additional basis set corrections, in order to obtain results close to the complete basis set limit. These reference data are used to benchmark a series of 12 excited-state wave function methods accounting for double and triple contributions, namely ADC(2), ADC(3), CIS(D), CIS(D), CC2, STEOM-CCSD, CCSD, CCSDR(3), CCSDT-3, CC3, CCSDT., and CCSDTQ. It turns out that CCSDTQ yields a negligible difference with the extrapolated CI values with a mean absolute error as small as 0.01 eV, whereas the coupled cluster approaches including iterative triples are also very accurate (mean absolute error of 0.03 eV). Consequently, CCSDT-3 and CC3 can be used to define reliable benchmarks. This observation does not hold for ADC(3) that delivers quite large errors for this set of small compounds, with a clear tendency to overcorrect its second-order version, ADC(2). Finally, we discuss the possibility to use basis set extrapolation approaches so as to tackle more easily larger compounds. \ No newline at end of file diff --git a/static/img/montain.jpeg b/static/data/publis/10/1021/acs/jctc/8b00406/picture.jpeg similarity index 100% rename from static/img/montain.jpeg rename to static/data/publis/10/1021/acs/jctc/8b00406/picture.jpeg diff --git a/static/data/publis/10/1021/acs/jctc/8b01205/abstract.html b/static/data/publis/10/1021/acs/jctc/8b01205/abstract.html new file mode 100644 index 00000000..2350514a --- /dev/null +++ b/static/data/publis/10/1021/acs/jctc/8b01205/abstract.html @@ -0,0 +1 @@ +Excited states exhibiting double-excitation character are notoriously difficult to model using conventional single-reference methods, such as adiabatic time-dependent density functional theory (TD-DFT) or equation-of-motion coupled cluster (EOM-CC). In addition, these states are typical experimentally “dark”, making their detection in photoabsorption spectra very challenging. Nonetheless, they play a key role in the faithful description of many physical, chemical, and biological processes. In the present work, we provide accurate reference excitation energies for transitions involving a substantial amount of double excitation using a series of increasingly large diffuse-containing atomic basis sets. Our set gathers 20 vertical transitions from 14 small- and medium-size molecules (acrolein, benzene, beryllium atom, butadiene, carbon dimer and trimer, ethylene, formaldehyde, glyoxal, hexatriene, nitrosomethane, nitroxyl, pyrazine, and tetrazine). Depending on the size of the molecule, selected configuration interaction (sCI) and/or multiconfigurational (CASSCF, CASPT2, (X)MS-CASPT2, and NEVPT2) calculations are performed in order to obtain reliable estimates of the vertical transition energies. In addition, coupled cluster approaches including at least contributions from iterative triples (such as CC3, CCSDT, CCSDTQ, and CCSDTQP) are assessed. Our results clearly evidence that the error in CC methods is intimately related to the amount of double-excitation character of the transition. For “pure” double excitations (i.e., for transitions which do not mix with single excitations), the error in CC3 can easily reach 1 eV, while it goes down to a few tenths of an electronvolt for more common transitions (such as in trans-butadiene) involving a significant amount of singles. As expected, CC approaches including quadruples yield highly accurate results for any type of transition. The quality of the excitation energies obtained with multiconfigurational methods is harder to predict. We have found that the overall accuracy of these methods is highly dependent on both the system and the selected active space. The inclusion of the σ and σ* orbitals in the active space, even for transitions involving mostly π and π* orbitals, is mandatory in order to reach high accuracy. A theoretical best estimate (TBE) is reported for each transition. 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z#_t>{CXo6f2VWbt1yMKq}Z$4skK(oS}4C}{C*M#_bo3rf@?{P z3@hbWeC_{PO!B`TK4vL3t%FSS-oxxYAKy0>3bS_+9dgV1ye$ZuuKhW=I6>?v<{$gc zF;y<{@JUo7o3;hB^X5y1R8=q5l6z#w=LceKicv=2mquq3mYYnSoDXHu>u6kZAY#^Y zt%NIf)*$!oeM%8?yYW^(M!xiVR9=DGjTmt!vr`b%%qZ8hCWL`&iAUQeU>gxCID<}0hJU`2a_L5#>UF6>sAzfuh*%L6)mvT4DWIi5L#04w0u8*GGYr= zb@V|=aNeM@Mb(rt^MrqYC%wB1@|N3!*#J%=`bxbdxkyZpG;O8f2L1RECqC3ND z@_raqr#)vmWYgp`n?<-ZjUIgs=*3KzkuBXo7$3*(XH%$8#26LWK|=EBLjA+dMMs@2T2Following our previous work focusing on compounds containing up to 3 non-hydrogen atoms [J. Chem. Theory Comput.2018, 14, 4360–4379], we present here highly accurate vertical transition energies obtained for 27 molecules encompassing 4, 5, and 6 non-hydrogen atoms: acetone, acrolein, benzene, butadiene, cyanoacetylene, cyanoformaldehyde, cyanogen, cyclopentadiene, cyclopropenone, cyclopropenethione, diacetylene, furan, glyoxal, imidazole, isobutene, methylenecyclopropene, propynal, pyrazine, pyridazine, pyridine, pyrimidine, pyrrole, tetrazine, thioacetone, thiophene, thiopropynal, and triazine. To obtain these energies, we use equation-of-motion/linear-response coupled cluster theory up to the highest technically possible excitation order for these systems (CC3, EOM-CCSDT, and EOM-CCSDTQ) and selected configuration interaction (SCI) calculations (with tens of millions of determinants in the reference space), as well as the multiconfigurational n-electron valence state perturbation theory (NEVPT2) method. All these approaches are applied in combination with diffuse-containing atomic basis sets. For all transitions, we report at least CC3/aug-cc-pVQZ vertical excitation energies as well as CC3/aug-cc-pVTZ oscillator strengths for each dipole-allowed transition. We show that CC3 almost systematically delivers transition energies in agreement with higher-level methods with a typical deviation of ±0.04 eV, except for transitions with a dominant double excitation character where the error is much larger. The present contribution gathers a large, diverse, and accurate set of more than 200 highly accurate transition energies for states of various natures (valence, Rydberg, singlet, triplet, n → π*, π → π*, ...). We use this series of theoretical best estimates to benchmark a series of popular methods for excited state calculations: CIS(D), ADC(2), CC2, STEOM-CCSD, EOM-CCSD, CCSDR(3), CCSDT-3, CC3, and NEVPT2. The results of these benchmarks are compared to the available literature data.

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the successive steps that made it possible to obtain increasingly accurate excitation energies with computational chemistry tools, eventually leading to chemically accurate vertical transition energies for small- and medium-size molecules. First, we describe the evolution of ab initio methods employed to define benchmark values, with the original Roos CASPT2 method, then the CC3 method as in the renowned Thiel set, and more recently the resurgence of selected configuration interaction methods. The latter method has been able to deliver consistently, for both single and double excitations, highly accurate excitation energies for small molecules, as well as medium-size molecules with compact basis sets. Second, we describe how these high-level methods and the creation of representative benchmark sets of excitation energies have allowed the fair and accurate assessment of the performance of computationally lighter methods. We conclude by discussing possible future theoretical and technological developments in the field. \ No newline at end of file diff --git a/static/data/publis/10/1021/acs/jpclett/0c00014/picture.jpeg b/static/data/publis/10/1021/acs/jpclett/0c00014/picture.jpeg new file mode 100644 index 0000000000000000000000000000000000000000..2398ca993ae84b98975e3726c78321f09a577de0 GIT binary patch literal 118884 zcmeFabwE^4+c$oe6e&qXIuwxZ29@sa5|*WQ*@fLD1OXF+MnP!_=}-`mR#Z>{k?s-! zX;ebV-&u^Wa(jE<&-1?T?=KJR*|}n_x#lx7*NK_4XSZ*63^=5vrl|%%z>Ocm4*EXW|lF%2+SV@DJUv8SPl#KK@mZx5URm&Sc7BhWaSaxbs3n;%Z& zv>O(e2Pgh&6Nc7v@PL`9T9|;WuZ4ZhV1P!UoQ+{vZ%=(kcPJ<%0}KE(fCB%V0XD!G zfB{&*8}P)L0uFlq&<3eJGp7+)(4Osr?lVIh+YR0dV(E zjj4aCvA!qP4TZ#j^20byWlt>fdnLe1I--9NMlKlLAA~X*sr(Ot#QsC*I3h4VBzi7b zpC5#(2SVis0pj?N>C;fS%Qqmtq68SJpH>FF!N<8|rHy?g|4N z7wn;KNSE*MQQ!ndpiie!SS-o|fkL``%R=^Df^*>~KKXaPk(-O_&jQl#0?@Y~`na)z zzwp%u+(-j^9XRH`e(#N=<9jlSz5U)!={)eYzme~e1mNCkPm|#X&9Z0p(;iK-w+DBS zyAb1mAZ*@o;)L{a?4A6n+T)2@C+z8-a^oc;JV~5#^0^!t5KD 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100644 --- a/static/js/createPubliUI.js +++ b/static/js/createPubliUI.js @@ -1,4 +1,8 @@ -function createPubliUI(publi,sets=new Map(),toolTips=false) { +function getPubliSubDir(DOI) { + return DOI.split(".").join("/") +} + +async function createPubliUI(publi,sets=new Map(),toolTips=false,abstract=false) { const art = $("
").addClass("publi") art.className = "publi" if (sets.has(publi.DOI) && sets.get(publi.DOI)!==null) { @@ -68,5 +72,16 @@ function createPubliUI(publi,sets=new Map(),toolTips=false) { month: "short", year: "numeric" }))).appendTo(art) + if (abstract) { + const dir = "/data/publis/"+getPubliSubDir(publi.DOI) + var ab = $("
",{id: "abstract",}).addClass("well").addClass("abstract") + var abfig =$("
").addClass("picture") + abfig.appendTo(ab) + $("",{src:dir+"/picture.jpeg"}).appendTo(abfig) + var htmltxt =await getTextFromFileUrlAsync(dir+"/abstract.html") + abtxt=$("

").html(htmltxt) + abtxt.appendTo(ab) + art.append(ab) + } return art } \ No newline at end of file diff --git a/static/js/getPublis.js b/static/js/getPublis.js index c6f0cfc7..acd05875 100644 --- a/static/js/getPublis.js +++ b/static/js/getPublis.js @@ -1,5 +1,5 @@ async function getPublis() { - const text = await getTextFromFileUrlAsync("/data/publis.yaml") + const text = await getTextFromFileUrlAsync("/data/publis/index.yaml") const myYaml=jsyaml.load(text); myYaml.sets= ((myYaml.sets===null) ? new Map() : new Map(Object.entries(myYaml.sets))); myYaml.others=((myYaml.others===null) ? new Map() : new Map(Object.entries(myYaml.others)));