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qp2/plugins/local/tc_bi_ortho/spin_mulliken.irp.f

115 lines
3.3 KiB
Fortran

BEGIN_PROVIDER [double precision, tc_spin_population, (ao_num,ao_num,N_states)]
implicit none
integer :: i,j,istate
BEGIN_DOC
! spin population on the ao basis :
! tc_spin_population(i,j) = rho_AO(alpha)(i,j) - rho_AO(beta)(i,j) * <AO_i|AO_j>
END_DOC
tc_spin_population = 0.d0
if(only_spin_tc_right)then
do i = 1, ao_num
do j = 1, ao_num
tc_spin_population(j,i,1) = tc_spin_dens_right_only(j,i) * ao_overlap(j,i)
enddo
enddo
else
do istate = 1, N_states
do i = 1, ao_num
do j = 1, ao_num
tc_spin_population(j,i,istate) = tc_spin_transition_matrix_ao(j,i,istate,istate) * ao_overlap(j,i)
enddo
enddo
enddo
endif
END_PROVIDER
BEGIN_PROVIDER [double precision, tc_spin_population_angular_momentum, (0:ao_l_max,N_states)]
&BEGIN_PROVIDER [double precision, tc_spin_population_angular_momentum_per_atom, (0:ao_l_max,nucl_num,N_states)]
implicit none
integer :: i,istate
double precision :: accu
tc_spin_population_angular_momentum = 0.d0
tc_spin_population_angular_momentum_per_atom = 0.d0
do istate = 1, N_states
do i = 1, ao_num
tc_spin_population_angular_momentum(ao_l(i),istate) += tc_spin_gross_orbital_product(i,istate)
tc_spin_population_angular_momentum_per_atom(ao_l(i),ao_nucl(i),istate) += tc_spin_gross_orbital_product(i,istate)
enddo
enddo
END_PROVIDER
BEGIN_PROVIDER [double precision, tc_spin_gross_orbital_product, (ao_num,N_states)]
implicit none
tc_spin_gross_orbital_product = 0.d0
integer :: i,j,istate
BEGIN_DOC
! gross orbital product for the spin population
END_DOC
do istate = 1, N_states
do i = 1, ao_num
do j = 1, ao_num
tc_spin_gross_orbital_product(i,istate) += tc_spin_population(j,i,istate)
enddo
enddo
enddo
END_PROVIDER
BEGIN_PROVIDER [double precision, tc_mulliken_spin_densities, (nucl_num,N_states)]
implicit none
integer :: i,j,istate
BEGIN_DOC
!ATOMIC SPIN POPULATION (ALPHA MINUS BETA)
END_DOC
tc_mulliken_spin_densities = 0.d0
do istate = 1, N_states
do i = 1, ao_num
tc_mulliken_spin_densities(ao_nucl(i),istate) += tc_spin_gross_orbital_product(i,istate)
enddo
enddo
END_PROVIDER
subroutine tc_print_mulliken_sd
implicit none
double precision :: accu
integer :: i
integer :: j
print*,'Mulliken spin densities'
accu= 0.d0
do i = 1, nucl_num
print*,i,nucl_charge(i),tc_mulliken_spin_densities(i,1)
accu += tc_mulliken_spin_densities(i,1)
enddo
print*,'Sum of Mulliken SD = ',accu
print*,'AO SPIN POPULATIONS'
accu = 0.d0
do i = 1, ao_num
accu += tc_spin_gross_orbital_product(i,1)
write(*,'(1X,I3,1X,A4,1X,I2,1X,A4,1X,F10.7)')i,trim(element_name(int(nucl_charge(ao_nucl(i))))),ao_nucl(i),trim(l_to_character(ao_l(i))),tc_spin_gross_orbital_product(i,1)
enddo
print*,'sum = ',accu
accu = 0.d0
print*,'Angular momentum analysis'
do i = 0, ao_l_max
accu += tc_spin_population_angular_momentum(i,1)
print*,' ',trim(l_to_character(i)),tc_spin_population_angular_momentum(i,1)
print*,'sum = ',accu
enddo
print*,'Angular momentum analysis per atom'
print*,'Angular momentum analysis'
do j = 1,nucl_num
accu = 0.d0
do i = 0, ao_l_max
accu += tc_spin_population_angular_momentum_per_atom(i,j,1)
write(*,'(1X,I3,1X,A4,1X,A4,1X,F10.7)')j,trim(element_name(int(nucl_charge(j)))),trim(l_to_character(i)),tc_spin_population_angular_momentum_per_atom(i,j,1)
print*,'sum = ',accu
enddo
enddo
end