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qp2/src/dft_utils_func/ecmd_pbe_general.irp.f
2020-04-23 12:42:06 +02:00

61 lines
2.1 KiB
Fortran

subroutine ec_md_pbe_on_top_general(mu,rho_a,rho_b,grad_rho_a,grad_rho_b,on_top,eps_c_md_on_top_PBE)
implicit none
BEGIN_DOC
!
! General e_cmd functional interpolating between :
!
! +) the large mu behaviour in cst/(\mu^3) on-top
!
! +) mu= 0 with the usal ec_pbe at
!
! Depends on : mu, the density (rho_a,rho_b), the square of the density gradient (grad_rho_a,grad_rho_b)
!
! the flavour of on-top densiyt (on_top) you fill in: in principle it should be the exact on-top
!
! The form of the functional was originally introduced in JCP, 150, 084103 1-10 (2019)
!
END_DOC
double precision, intent(in) :: mu,rho_a,rho_b,grad_rho_a(3),grad_rho_b(3),on_top
double precision, intent(out) :: eps_c_md_on_top_PBE
double precision :: pi, e_pbe,beta,denom
double precision :: grad_rho_a_2,grad_rho_b_2,grad_rho_a_b
double precision :: rhoc,rhoo,sigmacc,sigmaco,sigmaoo,vrhoc,vrhoo,vsigmacc,vsigmaco,vsigmaoo
integer :: m
pi = 4.d0 * datan(1.d0)
eps_c_md_on_top_PBE = 0.d0
! convertion from (alpha,beta) formalism to (closed, open) formalism for the density
call rho_ab_to_rho_oc(rho_a,rho_b,rhoo,rhoc)
if(rhoc.lt.1.d-10)then
return
else if(on_top/(rhoc**2) .lt. 1.d-6)then
return
endif
grad_rho_a_2 = 0.d0
grad_rho_b_2 = 0.d0
grad_rho_a_b = 0.d0
do m = 1, 3
grad_rho_a_2 += grad_rho_a(m)*grad_rho_a(m)
grad_rho_b_2 += grad_rho_b(m)*grad_rho_b(m)
grad_rho_a_b += grad_rho_a(m)*grad_rho_b(m)
enddo
! same same for gradients : convertion from (alpha,beta) formalism to (closed, open) formalism
call grad_rho_ab_to_grad_rho_oc(grad_rho_a_2,grad_rho_b_2,grad_rho_a_b,sigmaoo,sigmacc,sigmaco)
! usual PBE correlation energy using the density, spin polarization and density gradients for alpha/beta electrons
call ec_pbe_only(0.d0,rhoc,rhoo,sigmacc,sigmaco,sigmaoo,e_PBE)
denom = (-2.d0+sqrt(2d0))*sqrt(2.d0*pi)* on_top
if (dabs(denom) > 1.d-12) then
! quantity of Eq. (26)
beta = (3.d0*e_PBE)/denom
eps_c_md_on_top_PBE = e_PBE/(1.d0+beta*mu**3)
else
eps_c_md_on_top_PBE =0.d0
endif
end